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Simulating spin dynamics of supersolid states in a quantum Ising magnet

Motivated by a recent experimental study on the quantum Ising magnet $\text{K}_2\text{Co}(\text{SeO}_3)_2$ that presented spectroscopic evidence of zero-field supersolidity (Chen et al., arXiv:2402.15869), we simulate the excitation spectrum of the… Click to show full abstract

Motivated by a recent experimental study on the quantum Ising magnet $\text{K}_2\text{Co}(\text{SeO}_3)_2$ that presented spectroscopic evidence of zero-field supersolidity (Chen et al., arXiv:2402.15869), we simulate the excitation spectrum of the corresponding microscopic $XXZ$ model for the compound, using the recently developed excitation ansatz for infinite projected entangled-pair states. We map out the ground state phase diagram and compute the dynamical spin structure factors across a range of magnetic field strengths, focusing especially on the two supersolid phases found near zero and saturation fields. Our simulated excitation spectra for the zero-field supersolid"Y"phase are in excellent agreement with the experimental data - recovering the low-energy branches and integer quantized excited energy levels $\omega_n=nJ_{zz}$. Furthermore, we demonstrate the nonlocal multi-spin-flip features for modes at $\omega_2$, indicative of their multi-magnon nature. Additionally, we identify characteristics of the high-field supersolid"$\Psi$"phase in the simulated spectra, which should be compared with future experimental results.

Keywords: quantum ising; ising magnet; simulating spin; field

Journal Title: Physical Review B
Year Published: 2024

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