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Interplay of magnetism and superconductivity in the compressed Fe-ladder compound BaFe 2 Se 3

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High pressure resistance, susceptibility, and Fe $K\ensuremath{\beta}$ x-ray emission spectroscopy measurements were performed on Fe-ladder compound ${\mathrm{BaFe}}_{2}{\mathrm{Se}}_{3}$. Pressure-induced superconductivity was observed which is similar to the previously reported superconductivity in… Click to show full abstract

High pressure resistance, susceptibility, and Fe $K\ensuremath{\beta}$ x-ray emission spectroscopy measurements were performed on Fe-ladder compound ${\mathrm{BaFe}}_{2}{\mathrm{Se}}_{3}$. Pressure-induced superconductivity was observed which is similar to the previously reported superconductivity in the ${\mathrm{BaFe}}_{2}{\mathrm{S}}_{3}$ samples. The slope of local magnetic moment versus pressure shows an anomaly across the insulator-metal transition pressure in the ${\mathrm{BaFe}}_{2}{\mathrm{Se}}_{3}$ samples. The local magnetic moment is continuously decreasing with increasing pressure, and the superconductivity appears only when the local magnetic moment value is comparable to the one in the iron-pnictide superconductors. Our results indicate that the compressed ${\mathrm{BaFe}}_{2}C{h}_{3}$ ($Ch=\mathrm{S}$, Se) is a new family of iron-based superconductors. Despite the crystal structures completely different from the known iron-based superconducting materials, the magnetism in this Fe-ladder material plays a critical role in superconductivity. This behavior is similar to the other members of iron-based superconducting materials.

Keywords: pressure; ladder compound; mathrm; bafe mathrm; mathrm bafe; superconductivity

Journal Title: Physical Review B
Year Published: 2017

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