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Phonon Spectroscopy with Chirped Shear and Compressive Acoustic Pulses.

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Picosecond duration compressive and shear phonon wave packets injected into (311) GaAs slabs transform after propagation through ∼1  mm into chirped acoustic pulses with a frequency increasing in time due to… Click to show full abstract

Picosecond duration compressive and shear phonon wave packets injected into (311) GaAs slabs transform after propagation through ∼1  mm into chirped acoustic pulses with a frequency increasing in time due to phonon dispersion. By probing the temporal optical response to coherent phonons in a near surface layer of the GaAs slab, we show that phonon chirping opens a transformational route for high-sensitivity terahertz and subterahertz phonon spectroscopy. Temporal gating of the chirped phonon pulse allows the selection of a narrow band phonon spectrum with a central frequency up to 0.4 THz for longitudinal and 0.2 THz for transverse phonons.

Keywords: phonon; spectroscopy chirped; chirped shear; spectroscopy; phonon spectroscopy; acoustic pulses

Journal Title: Physical review letters
Year Published: 2017

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