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Quantum Criticality of an Ising-like Spin-1/2 Antiferromagnetic Chain in a Transverse Magnetic Field.

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We report on magnetization, sound-velocity, and magnetocaloric-effect measurements of the Ising-like spin-1/2 antiferromagnetic chain system BaCo_{2}V_{2}O_{8} as a function of temperature down to 1.3 K and an applied transverse magnetic field… Click to show full abstract

We report on magnetization, sound-velocity, and magnetocaloric-effect measurements of the Ising-like spin-1/2 antiferromagnetic chain system BaCo_{2}V_{2}O_{8} as a function of temperature down to 1.3 K and an applied transverse magnetic field up to 60 T. While across the Néel temperature of T_{N}∼5  K anomalies in magnetization and sound velocity confirm the antiferromagnetic ordering transition, at the lowest temperature the field-dependent measurements reveal a sharp softening of sound velocity v(B) and a clear minimum of temperature T(B) at B_{⊥}^{c,3D}=21.4  T, indicating the suppression of the antiferromagnetic order. At higher fields, the T(B) curve shows a broad minimum at B_{⊥}^{c}=40  T, accompanied by a broad minimum in the sound velocity and a saturationlike magnetization. These features signal a quantum phase transition, which is further characterized by the divergent behavior of the Grüneisen parameter Γ_{B}∝(B-B_{⊥}^{c})^{-1}. By contrast, around the critical field, the Grüneisen parameter converges as temperature decreases, pointing to a quantum critical point of the one-dimensional transverse-field Ising model.

Keywords: like spin; field; ising like; spin antiferromagnetic; antiferromagnetic chain; sound velocity

Journal Title: Physical review letters
Year Published: 2018

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