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X-ray absorption spectroscopy was used to probe the interactions between an octadentate hydroxypyridinone chelator and two transuranic elements in microgram quantities – plutonium and berkelium – within buffered solutions. Despite… Click to show full abstract
X-ray absorption spectroscopy was used to probe the interactions between an octadentate hydroxypyridinone chelator and two transuranic elements in microgram quantities – plutonium and berkelium – within buffered solutions. Despite the precedence for chelation-driven stabilization of the tetravalent oxidation state of actinides with this ligand, in situ reductive decomposition yielded plutonium(III) and berkelium(III) coordination complexes.
Keywords:
coordination complexes;
reduction route;
beam reduction;
situ beam;
hydroxypyridinone
Journal Title: Journal of Synchrotron Radiation
Year Published: 2022
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Journal Title: Journal of Synchrotron Radiation
Year Published: 2022
Link to full text (if available)
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recommendations!