Organo-halide Perovskite Solar Cells (PSC) have been reported to achieve remarkably high power conversion efficiency (PCE). A thorough understanding of the role of each component in solar cells and their… Click to show full abstract
Organo-halide Perovskite Solar Cells (PSC) have been reported to achieve remarkably high power conversion efficiency (PCE). A thorough understanding of the role of each component in solar cells and their effect as a whole is still required for further improvement in PCE. In this paper, the effect of Molybdenum Disulfide (MoS 2 ) in PSC with mesoporous structure configuration was analyzed using Solar Cell Capacitance Simulator (SCAPS). With the MoS 2 layer which having two-fold function, acting as a protective layer, by preventing the formation of shunt contacts between perovskite and Au electrode, and as a hole transport material (HTM) from the perovskite to the Spiro-OMETAD. As simulated, PSC demonstrates a PCE, ŋ of 13.1%, along with stability compared to typical structure of PSC without MoS 2 (Δ ŋ/ŋ=-9% vs. Δ ŋ/ŋ=-6%). The results pave the way towards the implementation of MoS 2 as a material able to boost shelf life which very useful for new material choice and optimization of HTMs.
               
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