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Strongly coupled exciton-surface plasmon polariton from excited-subband transitions of single-walled carbon nanotubes.

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We report experimental observation of strong coupling between surface plasmon polariton (SPP) propagating on a thin silver film and excitons from excited-subband transtitions of single-walled carbon nanotubes (SWNTs). Clear anti-crossing… Click to show full abstract

We report experimental observation of strong coupling between surface plasmon polariton (SPP) propagating on a thin silver film and excitons from excited-subband transtitions of single-walled carbon nanotubes (SWNTs). Clear anti-crossing behaviors were observed from attenuated total reflection measurements when the SPP energy approaches the 2nd subband transition of (6,5) SWNTs. The maximum Rabi splitting of the plasmon-exciton mixed states was extracted to be up to ~166.2 meV. Moreover, the splitting was found to be dependent linearly on the square root of the SWNTs concentration, in good agreement with theoretical prediction.

Keywords: subband; walled carbon; excited subband; single walled; surface plasmon; plasmon polariton

Journal Title: Optics express
Year Published: 2017

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