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Determining the absolute temporal field of ultra-broadband terahertz-infrared pulses with field-induced second-harmonic spectrograms.

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We demonstrate the use of spectrograms of the field-induced second-harmonic (FISH) signal generated in ambient air, to reconstruct the absolute temporal electric field of ultra-broadband terahertz-infrared (THz-IR) pulses with bandwidths… Click to show full abstract

We demonstrate the use of spectrograms of the field-induced second-harmonic (FISH) signal generated in ambient air, to reconstruct the absolute temporal electric field of ultra-broadband terahertz-infrared (THz-IR) pulses with bandwidths exceeding 100 THz. The approach is applicable even with relatively long (150-femtosecond) optical detection pulses, where the relative intensity and phase can be extracted from the moments of the spectrogram, as demonstrated by transmission spectroscopy of very thin samples. Auxiliary EFISH/ABCD measurements are used to provide the absolute field and phase calibration, respectively. We take into account the beam-shape/propagation effects about the detection focus on the measured FISH signals, which affect the field calibration, and show how an analysis of a set of measurements vs. truncation of the unfocused THz-IR beam can be used to correct for these. This approach could also be applied to the field calibration of ABCD measurements of conventional THz pulses.

Keywords: field induced; induced second; second harmonic; field; field ultra; absolute temporal

Journal Title: Optics express
Year Published: 2023

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