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Infrared spectral soot emission for robust and high-fidelity flame thermometry.

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Spectral soot emission (SSE) in the visible spectrum is a popular technique for non-intrusive thermometry in sooting flames. However, its accuracy is restricted by uncertainties in the wavelength dependence of… Click to show full abstract

Spectral soot emission (SSE) in the visible spectrum is a popular technique for non-intrusive thermometry in sooting flames. However, its accuracy is restricted by uncertainties in the wavelength dependence of soot optical properties. We propose a novel infrared spectral soot emission method that successfully addresses this issue. Comprehensive light extinction experiments were firstly conducted to explore the spectral variation of soot optical property. The results indicated a wavelength independence of the soot absorption function provided the wavelength of the incident light is larger than 1000 nm, thereby indicating through the Kirchhoff law the potential of a robust thermometry using infrared (>1000 nm) spectral soot emissions. Proof-of-concept experiments were performed for sooting premixed flames of ethylene with different equivalence ratios. The results demonstrated that the new method provided more accurate temperature results compared with its visible-NIR counterpart, particularly at flame positions where nascent soot particles are present. The proposed method is, to our knowledge, the first infrared spectral soot emission-based thermometry, and is believed to offer a solution to improving the fidelity of SSE with a cost-effective optical setup.

Keywords: infrared spectral; thermometry; spectral soot; soot emission; soot

Journal Title: Optics letters
Year Published: 2023

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