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Atomically Surficial Modulation in Two-Dimensional Semiconductor Nanocrystals for Selective Photocatalytic Reactions

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Photocatalysis, directly converting solar energy into chemical energy, is identified as an ideal strategy to reduce the increasing consumption of fossil fuels and facilitate carbon neutralization. In the past few… Click to show full abstract

Photocatalysis, directly converting solar energy into chemical energy, is identified as an ideal strategy to reduce the increasing consumption of fossil fuels and facilitate carbon neutralization. In the past few years, a great number of endeavors have been devoted to developing photocatalysts with a high conversion efficiency and selectivity. Atomically surficial modulation strategies, including surface vacancies, single-atom modification, and dual-site components, exhibited positive impacts on tuning key steps of photocatalytic reactions. In this mini-review, we focus on the latest progress of the atomically surficial modulations on two-dimensional semiconductor photocatalysts and their role in enhancing selectively photocatalytic performance. We hope that this mini-review could provide new insights for researchers on nanosynthesis and photocatalysis.

Keywords: two dimensional; atomically surficial; surficial modulation; photocatalytic reactions; dimensional semiconductor

Journal Title: Frontiers in Chemistry
Year Published: 2022

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