LAUSR

The Marangoni effect has been applied in the preparation of large-area ultrathin films. However, defects occur frequently during the transfer progress of ultrathin films to substrates, which limits its application in scalable and massive fabrication. Carbon nanotubes (CNTs), as typical one-dimensional carbon materials, are widely used in wearable and flexible sensors due to their outstanding electrical and mechanical properties. In this paper, Marangoni-driven self-assembled CNTs film was obtained by injecting 0.5 mL 1 mg·mL−1 CNTs/ethanol dispersion on 100 cm2 water dropwise; the thickness, sheet resistance, and optical transmittance (at 550 nm) of the as-prepared ultrathin film were 38 nm, 7.3 kΩ/□, and 66.9%, respectively. The CNTs film was transferred onto polydimethylsiloxane (PDMS) to prepare a conductive composite of CNTs/PDMS film and the sheet resistance of the composite film reached 21.0 kΩ/□. Furthermore, the packaged PDMS/CNTs/PDMS (PCP) strain sensors with a sandwich-like structure exhibited satisfactory sensitivity with a gauge factor of 3.4 at 50% strain, a large working range (89%), and excellent stability (>8000 cycles). The easy-making and low-cost sensors show great potential in wearable electronics, real-time motion detection, and electronic skin.