LAUSR

First, nickel particles were deposited on the surface of graphite nanoplatelets to fabricate highly conductive GnPs@Ni core-shell structure hybrid fillers via electroplating. The modified GnPs were blended with polyphenylene sulfone via the solution blending method, followed by the hot-pressing method to achieve high thermally conducting GnPs@Ni/PPSU composites for high performance electromagnetic interference effectiveness. The results showed that in-plane and through-plane thermal conductivity of the composite at the 40 wt% filler loading could reach 2.6 Wm−1K−1 and 3.7 Wm−1K−1, respectively, which were 9.4 and 20 times higher than that of pure PPSU resin. The orientation degree of fillers was discussed by XRD and SEM. Then, heat conduction data were fitted and analyzed by the Agari model, and the heat conduction mechanism was further explored. The testing results also demonstrated that the material exhibited good conductivity, electromagnetic shielding effectiveness and superior thermal stability. Overall, the GnPs@Ni/PPSU composites had high thermal conductivity and were effective electromagnetic shielding materials at high temperatures.