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GdV6Sn6: A Multi-carrier Metal with Non-magnetic 3d-electron Kagome Bands and 4f-electron Magnetism

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Electronic properties of the single crystal of GdV6Sn6, where non-magnetic V-kagome layers are separated by magnetic Gd-triangular lattice, are investigated. GdV6Sn6 exhibits unique magnetotransport properties at low-temperature such as non-linear… Click to show full abstract

Electronic properties of the single crystal of GdV6Sn6, where non-magnetic V-kagome layers are separated by magnetic Gd-triangular lattice, are investigated. GdV6Sn6 exhibits unique magnetotransport properties at low-temperature such as non-linear Hall resistivity and increase of resistance R in magnetic field H as R ~ H up to 56 T with Shubnikov–De Haas oscillations. Investigation of the non-magnetic analogue YV6Sn6 and the first principles calculations reveal these properties are relevant to the bands arising from the V-kagome layer. A magnetic transition at 5 K in GdV6Sn6 modifies the transport properties, pointing to a coupling between Gd-spins on the triangular lattice and carriers in the V-kagome layer.

Keywords: kagome; multi carrier; gdv6sn6; gdv6sn6 multi; non magnetic

Journal Title: Journal of the Physical Society of Japan
Year Published: 2021

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