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Published in 2023 at "ChemCatChem"
DOI: 10.1002/cctc.202300330
Abstract: NAD(P)+ regeneration is of great importance for dehydrogenase (DH)‐catalyzed oxidations. In this work, we report horseradish peroxidase (HRP)‐catalyzed aerobic oxidation of the reduced nicotinamide cofactors, including natural and non‐natural ones, into the oxidized form at…
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Keywords:
regeneration;
nicotinamide cofactors;
horseradish peroxidase;
promiscuity horseradish ... See more keywords
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Published in 2017 at "ChemSusChem"
DOI: 10.1002/cssc.201701288
Abstract: The catalytic promiscuity of hemoglobin (Hb) was explored for regenerating oxidized nicotinamide cofactors [NAD(P)+ ]. With H2 O2 as oxidant, Hb efficiently oxidized NAD(P)H into NAD(P)+ within 30 min. The new NAD(P)+ regeneration system was coupled…
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Keywords:
catalytic promiscuity;
catalyzed oxidation;
dehydrogenase catalyzed;
oxidation ... See more keywords
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Published in 2017 at "Current opinion in chemical biology"
DOI: 10.1016/j.cbpa.2017.02.021
Abstract: The view of enzymes as punctilious catalysts has been shifting as examples of their promiscuous behavior increase. However, unlike a number of cases where the physiological relevance of breached substrate specificity is questionable, the very…
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Keywords:
promiscuity;
promiscuity heme;
catalytic promiscuity;
synthesis ... See more keywords
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Published in 2020 at "Inorganica Chimica Acta"
DOI: 10.1016/j.ica.2020.119480
Abstract: Abstract A flexible single-side Mannich base ligand namely 4-(tert-butyl)-2-((ethyl(2-hydroxyethyl)amino)methyl)phenol (H2L) having O, N, O donor sites has been designed and synthesized using 4-(tert-butyl)phenol, formaldehyde and 2-(ethylamino)ethanol as precursors with the view to prepare polynuclear complex(s).…
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Keywords:
mannich base;
copper;
complex;
tert butyl ... See more keywords
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Published in 2019 at "Nature Reviews Chemistry"
DOI: 10.1038/s41570-019-0143-x
Abstract: The ability of one enzyme to catalyse multiple, mechanistically distinct transformations likely played a crucial role in organisms’ abilities to adapt to changing external stimuli in the past and can still be observed in extant…
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Keywords:
importance catalytic;
evolution;
enzyme design;
promiscuity ... See more keywords