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Published in 2023 at "Organic letters"
DOI: 10.1021/acs.orglett.3c01452
Abstract: We report a selective and sustainable synthesis of substituted pyrazoles via an eco-friendly acceptorless dehydrogenative annulation (ADA) of greener alcohols, malononitrile, and various aromatic hydrazides by newly synthesized binuclear Ru(II) p-cymene complexes. A discrete set…
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Keywords:
dehydrogenative annulation;
synthesis substituted;
sustainable synthesis;
substituted pyrazoles ... See more keywords
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Published in 2017 at "Organic letters"
DOI: 10.1021/acs.orglett.7b00562
Abstract: The discovery of a direct method for the synthesis of three-ring heterocyclic carbazoles from unactivated arenes and anilides by a metal-free (organic) intermolecular dehydrogenative annulation reaction under ambient laboratory conditions is reported. Iodine(III) was used…
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Keywords:
dehydrogenative annulation;
organic intermolecular;
annulation reaction;
intermolecular dehydrogenative ... See more keywords
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Published in 2018 at "Nature Communications"
DOI: 10.1038/s41467-018-06020-8
Abstract: Dehydrogenative annulation reactions are among the most straightforward and efficient approach for the preparation of cyclic structures. However, the applications of this strategy for the synthesis of saturated heterocycles have been rare. In addition, reported…
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Keywords:
dehydrogenative annulation;
annulation;
synthesis saturated;
alkenes diols ... See more keywords
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2
Published in 2023 at "Green Chemistry"
DOI: 10.1039/d3gc01329d
Abstract: The dehydrogenative [4+2] annulation is a step and atom-economical way to construct benzo-fused six-membered ring which are prevalent in natural products, pharmaceuticals and agrochemicals. Traditional protocols often require C-H activation...
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Keywords:
dehydrogenative annulation;
light promoted;
annulation;
heterogeneous visible ... See more keywords