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   Articles with "multicarbon" as a keyword



Advancing CO2 Upgrading to Multicarbon Products: Synergies Between Photo/Electrochemical and Biological Conversion

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recommendations! Published in 2025 at "Advanced Functional Materials"

DOI: 10.1002/adfm.202513716

Abstract: While photo‐ and electrochemical CO2 reduction efficiently generate C1–C2 molecules (e.g., formate, carbon monoxide, methane, ethylene), their limited selectivity and kinetic constraints impede direct C2+ synthesis. Conversely, biological CO2 fixation excels at producing multicarbon compounds (e.g.,… read more here.

Keywords: co2 upgrading; co2; biological conversion; photo electrochemical ... See more keywords

Enhancing microbial CO2 electrocatalysis for multicarbon reduction in a wet amine-based catholyte.

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recommendations! Published in 2024 at "ChemSusChem"

DOI: 10.1002/cssc.202301342

Abstract: Microbial CO2 electroreduction (mCO2ER) offers a promising approach for producing high-value multicarbon reductants from CO2 by combining CO2 fixing microorganisms with conducting materials (i.e., cathodes). However, the solubility and availability of CO2 in an aqueous… read more here.

Keywords: catholyte; multicarbon; co2; amine based ... See more keywords

Porous Copper Microspheres for Selective Production of Multicarbon Fuels via CO2 Electroreduction.

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recommendations! Published in 2019 at "Small"

DOI: 10.1002/smll.201902582

Abstract: The electroreduction of carbon dioxide (CO2 ) toward high-value fuels can reduce the carbon footprint and store intermittent renewable energy. The iodide-ion-assisted synthesis of porous copper (P-Cu) microspheres with a moderate coordination number of 7.7,… read more here.

Keywords: porous copper; copper microspheres; co2; electroreduction ... See more keywords

Steering the Selectivity of Carbon Dioxide Electroreduction from Single-Carbon to Multicarbon Products on Metal-Organic Frameworks via Facet Engineering.

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recommendations! Published in 2024 at "Nano letters"

DOI: 10.1021/acs.nanolett.3c04092

Abstract: Although metal-organic frameworks (MOFs) have attracted more attention for the electrocatalytic CO2 reduction reaction (CO2RR), obtaining multicarbon products with a high Faradaic efficiency (FE) remains challenging, especially under neutral conditions. Here, we report the controlled… read more here.

Keywords: carbon; organic frameworks; single carbon; multicarbon products ... See more keywords

Constructing Favorable Microenvironment on Copper Grain Boundaries for CO2 Electro-conversion to Multicarbon Products.

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recommendations! Published in 2024 at "Nano letters"

DOI: 10.1021/acs.nanolett.4c02343

Abstract: The electrochemical CO2 reduction reaction (eCO2RR) to multicarbon chemicals provides a promising avenue for storing renewable energy. Herein, we synthesized small Cu nanoparticles featuring enriched tiny grain boundaries (RGBs-Cu) through spatial confinement and in situ… read more here.

Keywords: grain boundaries; favorable microenvironment; constructing favorable; multicarbon products ... See more keywords

NHC-CDI Ligands Boost Multicarbon Production in Electrocatalytic CO2 Reduction by Increasing Accumulated Charged Intermediates and Promoting *CO Dimerization on Cu.

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recommendations! Published in 2024 at "Journal of the American Chemical Society"

DOI: 10.1021/jacs.3c14306

Abstract: Copper-based materials exhibit significant potential as catalysts for electrochemical CO2 reduction, owing to their capacity to generate multicarbon hydrocarbons. The molecular functionalization of Cu electrodes represents a simple yet powerful strategy for improving the intrinsic… read more here.

Keywords: multicarbon product; co2 reduction; surface; multicarbon ... See more keywords

Selective electrochemical CO2 conversion to multicarbon alcohols on highly efficient N-doped porous carbon-supported Cu catalysts

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recommendations! Published in 2020 at "Green Chemistry"

DOI: 10.1039/c9gc03088c

Abstract: The selective and efficient electrocatalytic transformation of carbon dioxide (CO2) to multicarbon alcohols (e.g., C2H5OH and C3H7OH) is a challenge in renewable and sustainable energy research. Herein, a series of hybrid catalysts consisting of Cu… read more here.

Keywords: doped porous; porous carbon; co2; multicarbon alcohols ... See more keywords