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Published in 2022 at "Chemical reviews"
DOI: 10.1021/acs.chemrev.1c00929
Abstract: Proton-coupled electron transfer (PCET) plays an essential role in a wide range of electrocatalytic processes. A vast array of theoretical and computational methods have been developed to study electrochemical PCET. These methods can be used…
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Keywords:
coupled electron;
proton;
electron transfer;
proton coupled ... See more keywords
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Published in 2022 at "Inorganic chemistry"
DOI: 10.1021/acs.inorgchem.2c01930
Abstract: Molecular systems combining light harvesting and charge storage are receiving great attention in the context of, for example, artificial photosynthesis and solar fuel generation. As part of ongoing efforts to develop new concepts for photoinduced…
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Keywords:
bipyridine ligand;
state;
sulfurated bipyridine;
ligand ... See more keywords
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Published in 2022 at "Organic letters"
DOI: 10.1021/acs.orglett.2c00662
Abstract: Herein, we report the enantioselective addition of remote alkyl radicals, generated from the ring opening of unstrained cycloalkanols by a proton-coupled electron transfer (PCET) process, to 2-acyl imidazoles previously coordinated to a rhodium-based chiral Lewis…
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Keywords:
alkyl radicals;
addition remote;
remote alkyl;
enantioselective addition ... See more keywords
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Published in 2020 at "Molecules"
DOI: 10.3390/molecules25061443
Abstract: Recent experimental studies of kinetic isotope effects (KIE-s) and hydrogen tunnelling comprising three proton-coupled electron transfer (PCET) oxidations of ascorbate monoanion, (a) in aqueous reaction solutions, (b) in the mixed water-organic cosolvent systems, (c) in…
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Keywords:
isotope effects;
pcet;
chemistry;
kinetic isotope ... See more keywords