Articles with "single atoms" as a keyword



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Fe Isolated Single Atoms on S, N Codoped Carbon by Copolymer Pyrolysis Strategy for Highly Efficient Oxygen Reduction Reaction.

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Published in 2018 at "Advanced materials"

DOI: 10.1002/adma.201800588

Abstract: Heteroatom-doped Fe-NC catalyst has emerged as one of the most promising candidates to replace noble metal-based catalysts for highly efficient oxygen reduction reaction (ORR). However, delicate controls over their structure parameters to optimize the catalytic… read more here.

Keywords: single atoms; isolated single; efficient oxygen; codoped carbon ... See more keywords
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A General Method for Transition Metal Single Atoms Anchored on Honeycomb-Like Nitrogen-Doped Carbon Nanosheets.

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Published in 2020 at "Advanced materials"

DOI: 10.1002/adma.201906905

Abstract: Excavating and developing highly efficient and cost-effective nonnoble metal single-atom catalysts for electrocatalytic reactions is of paramount significance but still in its infancy. Herein, reported is a general NaCl template-assisted strategy for rationally designing and… read more here.

Keywords: hnc 500; metal single; transition metal; 500 850 ... See more keywords
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Integrating Single Atoms with Different Microenvironments into One Porous Organic Polymer for Efficient Photocatalytic CO2 Reduction.

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Published in 2021 at "Advanced materials"

DOI: 10.1002/adma.202101568

Abstract: The precise identification of single-atom catalysts (SACs) activity and boosting their efficiency toward CO2 conversion is imperative yet quite challenging. Herein, for the first time a series of porous organic polymers is designed and prepared… read more here.

Keywords: co2 reduction; integrating single; porous organic; single atoms ... See more keywords
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Synergy between Palladium Single Atoms and Nanoparticles via Hydrogen Spillover for Enhancing CO2 Photoreduction to CH4

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Published in 2022 at "Advanced Materials"

DOI: 10.1002/adma.202200057

Abstract: Selective photoreduction of carbon dioxide (CO2) into carbon‐neutral fuels such as methane (CH4) is extremely desirable but remains a challenge since sluggish multiple proton–electron coupling transfer and various C1 intermediates are involved. Herein, a synergistic… read more here.

Keywords: single atoms; ch4; hydrogen spillover; via hydrogen ... See more keywords
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Isolating Single and Few Atoms for Enhanced Catalysis

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Published in 2022 at "Advanced Materials"

DOI: 10.1002/adma.202201796

Abstract: Atomically dispersed metal catalysts have triggered great interest in the field of catalysis owing to their unique features. Isolated single or few metal atoms can be anchored on substrates via chemical bonding or space confinement… read more here.

Keywords: dacs atomic; catalysis; isolating single; single atoms ... See more keywords
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Vacancy‐Rich MXene‐Immobilized Ni Single Atoms as a High‐Performance Electrocatalyst for the Hydrazine Oxidation Reaction

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Published in 2022 at "Advanced Materials"

DOI: 10.1002/adma.202204388

Abstract: Single‐atom catalysts (SACs), on account of their outstanding catalytic potential, are currently emerging as high‐performance materials in the field of heterogeneous catalysis. Constructing a strong interaction between the single atom and its supporting matrix plays… read more here.

Keywords: single atoms; reaction; oxidation reaction; hydrazine oxidation ... See more keywords
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Regulating the Coordination Environment of Mesopore‐Confined Single Atoms from Metalloprotein‐MOFs for Highly Efficient Biocatalysis

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Published in 2022 at "Advanced Materials"

DOI: 10.1002/adma.202205674

Abstract: Single‐atom catalysts (SACs) exhibit unparalleled atomic utilization and catalytic efficiency, yet it is challenging to modulate SACs with highly dispersed single‐atoms, mesopores, and well‐regulated coordination environment simultaneously and ultimately maximize their catalytic efficiency. Here, a… read more here.

Keywords: single atoms; sacs; coordination; highly efficient ... See more keywords
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Strong Electronic Metal–Support Interaction between Iridium Single Atoms and a WO3 Support Promotes Highly Efficient and Robust CO2 Cycloaddition

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Published in 2022 at "Advanced Materials"

DOI: 10.1002/adma.202206991

Abstract: The carbon dioxide (CO2) cycloaddition of epoxides to cyclic carbonates is of great industrial importance owing to the high economical values of its products. Single‐atom catalysts (SACs) have great potential in CO2 cycloaddition by virtue… read more here.

Keywords: co2; co2 cycloaddition; single atoms; wo3 support ... See more keywords
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Modulating the Site Density of Mo Single Atoms to Catch Adventitious O Atoms for Efficient H2O2 Oxidation with Light

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Published in 2022 at "Advanced Materials"

DOI: 10.1002/adma.202208704

Abstract: Coordination environment and site density have great impacts on the catalytic performance for single atoms (SAs). Herein, the site density of Mo‐SAs on red polymeric carbon nitrides (RPCN) is modulated via a local carbonization strategy… read more here.

Keywords: oxidation; single atoms; catch adventitious; site ... See more keywords
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Pt Single Atoms on CrN Nanoparticles Deliver Outstanding Activity and CO Tolerance in the Hydrogen Oxidation Reaction

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Published in 2022 at "Advanced Materials"

DOI: 10.1002/adma.202208799

Abstract: The large‐scale application of proton exchange membrane fuel cells is currently hampered by high cost of commercial Pt catalysts and their susceptibility to poisoning by CO impurities in H2 feed. In this context, the development… read more here.

Keywords: oxidation reaction; hydrogen oxidation; sacs crn; single atoms ... See more keywords
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Dynamic Reconstitution Between Copper Single Atoms and Clusters for Electrocatalytic Urea Synthesis

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Published in 2023 at "Advanced Materials"

DOI: 10.1002/adma.202300020

Abstract: Electrocatalytic CN coupling between carbon dioxide and nitrate has emerged to meet the comprehensive demands of carbon footprint closing, valorization of waste, and sustainable manufacture of urea. However, the identification of catalytic active sites and… read more here.

Keywords: copper single; single atoms; synthesis; reconstitution copper ... See more keywords