Construction of Ultrathin S‐Scheme Heterojunctions of Single Ni Atom Immobilized Ti‐MOF and BiVO4 for CO2 Photoconversion of nearly 100% to CO by Pure Water
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DOI: 10.1002/adma.202205303
Abstract: To rationally design single‐atom metal–organic framework (MOF)‐involving photocatalysts remains an ongoing challenge for efficient CO2 conversion. Here, cuppy microstructures, consisting of a Ti(IV)‐oxo node and three linked carboxylic moieties, in the single‐coordination‐layer Ti2(H2dobdc)3 MOF (NTU‐9)… read more here.
Keywords: single sites; mof; single atom; mof bivo4 ... See more keywords
Nitrogen-coordinated single Fe sites for efficient electrocatalytic N2 fixation in neutral media
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DOI: 10.1016/j.nanoen.2019.04.092
Abstract: Abstract Electrocatalytic nitrogen reduction reaction (NRR) for NH3 generation under ambient conditions presents a promising alternative to the conventional Haber–Bosch process. Here, we report a Fe single-atom catalyst for ambient electrochemical NH3 synthesis. This catalyst… read more here.
Keywords: sites efficient; efficient electrocatalytic; coordinated single; nitrogen ... See more keywords
Encapsulation of Co single sites in covalent triazine frameworks for photocatalytic production of syngas
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DOI: 10.1016/s1872-2067(20)63603-8
Abstract: Abstract The photocatalytic production of syngas using a noble-metal-free catalytic system is a promising approach for renewable energy and environmental sustainability. In this study, we demonstrate an efficient catalytic system formed by integrating Co single… read more here.
Keywords: production syngas; production; single sites; sites covalent ... See more keywords
Integrating single Co sites into crystalline covalent triazine frameworks for photoreduction of CO2.
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DOI: 10.1039/d2cc02481k
Abstract: Bipyridine-containing covalent triazine framework (CTF-Bpy) was used to prove that the single site distribution of Co2+ was possible. The Co2+-loaded CTF-Bpy-Co produced 120 μmol CO with a selectivity of 83.8% over 10 h of irradiation… read more here.
Keywords: single sites; integrating single; sites crystalline; covalent triazine ... See more keywords