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Published in 2022 at "ChemistryOpen"
DOI: 10.1002/open.202200021
Abstract: Abstract Measuring the Lewis‐acidic surface sites in catalysis is problematic when the material‘s surface area is very low (SBET ≤1 m2 ⋅ g−1). For the first time, a quantitative assessment of total acidic surface sites of very small…
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Keywords:
lewis acidic;
molecule;
surface;
acidic surface ... See more keywords
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2
Published in 2021 at "ACS Central Science"
DOI: 10.1021/acscentsci.0c01486
Abstract: Increasing attention has been paid to single-atom catalysts (SACs) in heterogeneous catalysis because of their unique electronic properties, maximized atomic utilization efficiency, and potential to serve as a bridge between the heterogeneous and homogeneous catalysis.…
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Keywords:
fully exposed;
utilization efficiency;
surface sites;
exposed cluster ... See more keywords
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Published in 2020 at "ACS Nano"
DOI: 10.1021/acsnano.0c03004
Abstract: Metal nanoparticles are attractive for plasmon-enhanced generation of hot carriers, which may be harnessed in photochemical reactions. In this work, we analyze the coherent femtosecond dynamics of photon absorption, plasmon formation, and subsequent hot-carrier generation…
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Keywords:
carrier generation;
generation;
structure;
hot carrier ... See more keywords
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Published in 2018 at "Chemical communications"
DOI: 10.1039/c8cc08066f
Abstract: Low concentration tin bronze alloys show high selectivity for CO2 electroreduction to CO, while high concentration tin bronze alloys show high selectivity for formate. The tin surface sites appear to control selectivity by influencing the…
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Keywords:
co2;
surface sites;
bronze alloys;
tin surface ... See more keywords
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Published in 2021 at "Chemical Science"
DOI: 10.1039/d1sc02174e
Abstract: The experimentally validated computational models developed herein, for the first time, show that Mn-promotion does not enhance the activity of the surface Na2WO4 catalytic active sites for CH4 heterolytic dissociation during OCM. Contrary to previous…
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Keywords:
surface sites;
surface;
methane;
combined computational ... See more keywords
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2
Published in 2023 at "Chemical Science"
DOI: 10.1039/d2sc06827c
Abstract: The Union Carbide (UC) ethylene polymerization catalyst, based on silica-supported chromocene, is one of the first industrial catalysts prepared by surface organometallic chemistry, though the structure of the surface sites remains elusive. Recently, our group…
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Keywords:
polymerization catalyst;
surface;
chemical shifts;
surface sites ... See more keywords